Wang et al. 2020 - Jilin total diet study metals
Wang and colleagues measured lead, total arsenic, cadmium, and aluminum in Jilin Province total-diet-study food groups. The study compares Songhua River Basin and other-area composites and uses consumption data from 7700 residents to estimate dietary exposure. Arsenic occurrence values are total arsenic; the risk assessment conservatively evaluates total As as if it were inorganic As.
Key numbers
The abstract reports overall mean concentrations of 0.0189 mg/kg Pb, 0.0691 mg/kg As, 0.0085 mg/kg Cd, and 9.309 mg/kg Al across the total diet. Table 3 reports food-group means:
| Food group | Pb, mg/kg | tAs, mg/kg | Cd, mg/kg | Al, mg/kg |
|---|---|---|---|---|
| Cereals and cereal products | 0.008 | 0.024 | 0.004 | 44.016 |
| Beans, nuts, and their products | 0.045 | 0.020 | 0.024 | 3.480 |
| Potatoes and their products | 0.061 | 0.011 | 0.012 | 16.424 |
| Meat and its products | 0.038 | 0.018 | 0.008 | 4.485 |
| Eggs and egg products | 0.029 | 0.017 | 0.003 | 4.286 |
| Aquatic products | 0.030 | 0.728 | 0.005 | 4.235 |
| Milk and dairy products | 0.007 | 0.004 | 0.003 | 1.984 |
| Vegetables and vegetable products | 0.012 | 0.118 | 0.011 | 4.476 |
| Fruits and fruit products | 0.006 | 0.004 | 0.004 | 2.361 |
| Sugar and sugar products | 0.006 | 0.004 | 0.003 | 10.196 |
| Drinking water and beverages | 0.003 | 0.004 | 0.003 | 1.620 |
| Alcoholic drinks | 0.001 | 0.004 | 0.003 | 3.259 |
Table 2 and the results text identify the highest product-level concentrations:
| Analyte | Highest source category/product | Source-reported concentration |
|---|---|---|
| Pb | Potatoes and their products | 0.0610 mg/kg |
| Pb | Vermicelli within potatoes/products | 0.0697 mg/kg |
| tAs | Aquatic products and derivatives | 0.728 mg/kg |
| tAs | Cod within aquatic products | 1.403 mg/kg |
| Cd | Beans, nuts, and their products | 0.0240 mg/kg |
| Cd | Peanut within beans/nuts/products | 0.0841 mg/kg |
| Al | Cereals and cereal products | 44.016 mg/kg |
| Al | Deep-fried dough sticks | 250.120 mg/kg |
Table 5 reports mean dietary exposure:
| Population group | People | Pb, µg/kg bw | Pb MOE | tAs, µg/kg bw | As MOE | Cd, µg/kg bw | Cd PTMI, % | Al, µg/kg bw | Al PTWI, % |
|---|---|---|---|---|---|---|---|---|---|
| 2-6 years | 87 | 0.51 | 1.18 | 0.52 | 5.72 | 0.22 | 26.52 | 204.96 | 71.74 |
| 7-17 years | 450 | 0.34 | 3.53 | 0.39 | 7.69 | 0.13 | 15.10 | 162.03 | 56.71 |
| 18-40 years | 1774 | 0.32 | 3.73 | 0.33 | 9.19 | 0.11 | 12.99 | 119.25 | 41.74 |
| 41-65 years | 4146 | 0.19 | 6.26 | 0.25 | 11.87 | 0.08 | 9.89 | 113.60 | 39.76 |
| >65 years | 1243 | 0.26 | 4.66 | 0.26 | 11.71 | 0.07 | 8.70 | 94.62 | 33.12 |
| Overall population | 7700 | 0.32 | 3.71 | 0.35 | 8.57 | 0.12 | 14.64 | 138.89 | 48.61 |
The contribution analysis reports potatoes and their products as the main Pb exposure source at 24.89%, followed by beans/nuts/products at 17.21%. Aquatic products and derivatives contributed 52.14% of As exposure, vegetables and vegetable products contributed 31.3% of Cd exposure, and cereals and cereal products contributed 70.22% of Al exposure.
Methods (brief)
The study used a total diet study approach in which food groups were purchased, cooked or prepared according to local methods, homogenized, and analyzed as mixed-food samples. The 12 food groups included cereals, beans/nuts, potatoes, meat, eggs, aquatic products, milk/dairy, vegetables, fruits, sugar, drinking water/beverages, and alcoholic drinks. Solid samples of 0.3-0.5 g and liquid samples of 1.0 g were digested with nitric acid and analyzed by ICP-MS. The certified reference material GBW 10011 was used for quality control, with reported relative standard deviations of 4.51%-9.44%.
Implications
This source contributes China/Jilin total-diet occurrence and exposure context for Pb, total As, Cd, and Al across broad prepared-food groups. It is especially relevant for cereal/aluminum context and for distinguishing aquatic-product total-As occurrence from inorganic-arsenic evidence. The paper reports that deep-fried dough sticks exceeded the Chinese limit for aluminum in fried cereals, but it does not report brand-level results.
Verification notes
- PDF text extracted with
pdftotext -layout; title page, methods, Tables 2-6, and discussion were readable. - DOI
10.1002/fsn3.1851, raw handleMFK_wang2020, and cite-key checks found no existing source page before creation. - Table 3 means, Table 5 exposure values, and narrative product maxima were checked against the extracted text. Units are preserved as reported (
mg/kgfor concentrations andµg/kg bwfor exposure); no conversion was performed. - Speciation: arsenic was measured as total As. The authors state that total As was evaluated as inorganic As for a conservative risk assessment; this page keeps occurrence metals as
tAsand does not route the paper as measured iAs evidence. - Brand firewall: the source reports total-diet composite food/product groups, not brand-level values.
- The current product taxonomy snapshot does not list a dairy product slug; milk/dairy findings are represented in frontmatter only with the closed ingredient slug
[[ingredients/milk-and-dairy]]. Noodles are represented with the closed ingredient slug[[ingredients/noodles]]and routed through closed grain-product slugs rather than a nonexistentproducts/noodlesslug. - Frontmatter product and ingredient slugs were checked against
docs/gpt-collaboration/taxonomy-snapshot.md; no new product or ingredient slug was invented.
Page history
The five most recent substantive edits to this page. The full version history lives in git; when DOI minting comes online (see schema docs), each entry below will also link to a version-pinned DataCite DOI.
| Commit | Date | Description |
|---|---|---|
| 9792010 | 2026-06-08 | ingest: garrity1990-mt1-tissue-specific-promoter fresh from MFK/heavy_metals_peptides |