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Wang et al. 2020 - Jilin total diet study metals

Wang and colleagues measured lead, total arsenic, cadmium, and aluminum in Jilin Province total-diet-study food groups. The study compares Songhua River Basin and other-area composites and uses consumption data from 7700 residents to estimate dietary exposure. Arsenic occurrence values are total arsenic; the risk assessment conservatively evaluates total As as if it were inorganic As.

Key numbers

The abstract reports overall mean concentrations of 0.0189 mg/kg Pb, 0.0691 mg/kg As, 0.0085 mg/kg Cd, and 9.309 mg/kg Al across the total diet. Table 3 reports food-group means:

Food groupPb, mg/kgtAs, mg/kgCd, mg/kgAl, mg/kg
Cereals and cereal products0.0080.0240.00444.016
Beans, nuts, and their products0.0450.0200.0243.480
Potatoes and their products0.0610.0110.01216.424
Meat and its products0.0380.0180.0084.485
Eggs and egg products0.0290.0170.0034.286
Aquatic products0.0300.7280.0054.235
Milk and dairy products0.0070.0040.0031.984
Vegetables and vegetable products0.0120.1180.0114.476
Fruits and fruit products0.0060.0040.0042.361
Sugar and sugar products0.0060.0040.00310.196
Drinking water and beverages0.0030.0040.0031.620
Alcoholic drinks0.0010.0040.0033.259

Table 2 and the results text identify the highest product-level concentrations:

AnalyteHighest source category/productSource-reported concentration
PbPotatoes and their products0.0610 mg/kg
PbVermicelli within potatoes/products0.0697 mg/kg
tAsAquatic products and derivatives0.728 mg/kg
tAsCod within aquatic products1.403 mg/kg
CdBeans, nuts, and their products0.0240 mg/kg
CdPeanut within beans/nuts/products0.0841 mg/kg
AlCereals and cereal products44.016 mg/kg
AlDeep-fried dough sticks250.120 mg/kg

Table 5 reports mean dietary exposure:

Population groupPeoplePb, µg/kg bwPb MOEtAs, µg/kg bwAs MOECd, µg/kg bwCd PTMI, %Al, µg/kg bwAl PTWI, %
2-6 years870.511.180.525.720.2226.52204.9671.74
7-17 years4500.343.530.397.690.1315.10162.0356.71
18-40 years17740.323.730.339.190.1112.99119.2541.74
41-65 years41460.196.260.2511.870.089.89113.6039.76
>65 years12430.264.660.2611.710.078.7094.6233.12
Overall population77000.323.710.358.570.1214.64138.8948.61

The contribution analysis reports potatoes and their products as the main Pb exposure source at 24.89%, followed by beans/nuts/products at 17.21%. Aquatic products and derivatives contributed 52.14% of As exposure, vegetables and vegetable products contributed 31.3% of Cd exposure, and cereals and cereal products contributed 70.22% of Al exposure.

Methods (brief)

The study used a total diet study approach in which food groups were purchased, cooked or prepared according to local methods, homogenized, and analyzed as mixed-food samples. The 12 food groups included cereals, beans/nuts, potatoes, meat, eggs, aquatic products, milk/dairy, vegetables, fruits, sugar, drinking water/beverages, and alcoholic drinks. Solid samples of 0.3-0.5 g and liquid samples of 1.0 g were digested with nitric acid and analyzed by ICP-MS. The certified reference material GBW 10011 was used for quality control, with reported relative standard deviations of 4.51%-9.44%.

Implications

This source contributes China/Jilin total-diet occurrence and exposure context for Pb, total As, Cd, and Al across broad prepared-food groups. It is especially relevant for cereal/aluminum context and for distinguishing aquatic-product total-As occurrence from inorganic-arsenic evidence. The paper reports that deep-fried dough sticks exceeded the Chinese limit for aluminum in fried cereals, but it does not report brand-level results.

Verification notes

  • PDF text extracted with pdftotext -layout; title page, methods, Tables 2-6, and discussion were readable.
  • DOI 10.1002/fsn3.1851, raw handle MFK_wang2020, and cite-key checks found no existing source page before creation.
  • Table 3 means, Table 5 exposure values, and narrative product maxima were checked against the extracted text. Units are preserved as reported (mg/kg for concentrations and µg/kg bw for exposure); no conversion was performed.
  • Speciation: arsenic was measured as total As. The authors state that total As was evaluated as inorganic As for a conservative risk assessment; this page keeps occurrence metals as tAs and does not route the paper as measured iAs evidence.
  • Brand firewall: the source reports total-diet composite food/product groups, not brand-level values.
  • The current product taxonomy snapshot does not list a dairy product slug; milk/dairy findings are represented in frontmatter only with the closed ingredient slug [[ingredients/milk-and-dairy]]. Noodles are represented with the closed ingredient slug [[ingredients/noodles]] and routed through closed grain-product slugs rather than a nonexistent products/noodles slug.
  • Frontmatter product and ingredient slugs were checked against docs/gpt-collaboration/taxonomy-snapshot.md; no new product or ingredient slug was invented.

Page history

The five most recent substantive edits to this page. The full version history lives in git; when DOI minting comes online (see schema docs), each entry below will also link to a version-pinned DataCite DOI.

CommitDateDescription
97920102026-06-08ingest: garrity1990-mt1-tissue-specific-promoter fresh from MFK/heavy_metals_peptides