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Maduabuchi et al. 2007 — Arsenic and chromium in Nigerian beverages

Maduabuchi and colleagues measured arsenic and chromium in 50 canned and non-canned beverages purchased in Nigeria. The study digested beverage samples in nitric acid and quantified As and Cr by atomic absorption spectrophotometry. The occurrence finding is that both canned and non-canned beverage groups contained samples above the U.S. EPA drinking-water MCLs used as comparators by the authors; the paper does not perform arsenic or chromium speciation.

Key numbers

FindingSource-reported value
Total sample count50 beverage samples
Canned beverage count21
Non-canned beverage count29
Arsenic detection limit<DL is defined as value less than 0.001 mg/L
Chromium detection limit<DL is defined as value less than 0.001 mg/L
Canned beverage arsenic range0.003 to 0.161 mg/L
Non-canned beverage arsenic range0.002 to 0.261 mg/L
Canned beverage arsenic above source-used MCL33.3% exceeded 0.01 mg/L
Non-canned beverage arsenic above source-used MCL55.2% exceeded 0.01 mg/L
Combined arsenic exceedance46% of canned and non-canned beverages failed to meet the source-used U.S. EPA criterion
Canned beverage total chromium range0.04 to 0.59 mg/L
Non-canned beverage total chromium range0.01 to 0.55 mg/L
Canned beverage chromium above source-used MCL76.2% exceeded 0.10 mg/L
Non-canned beverage chromium above source-used MCL68.9% exceeded 0.10 mg/L
Combined chromium exceedance72% of canned and non-canned beverages failed to meet the source-used U.S. EPA criterion
Highest arsenic concentration in the study0.261 mg/L in the non-canned beverage group
Highest total chromium concentration in the study0.59 mg/L in the canned beverage group

The source tables provide drink-by-drink values and commercial product names. This page reports only aggregate canned/non-canned ranges and exceedance percentages to preserve the brand firewall.

Methods (brief)

Fifty beverage samples were purchased in Nigeria in March 2005, including 21 canned and 29 non-canned beverages. Five milliliters of each sample was digested with 15 mL nitric acid, made up to 50 mL with deionized water, heated until fully digested and reduced to 10 mL, cooled, and filtered. Arsenic and chromium were analyzed with a Unicam Atomic Absorption Spectrophotometer Model 929 using air-acetylene flame. Arsenic was analyzed at 193.7 nm; chromium was analyzed at 358 nm. Samples were analyzed in duplicates.

Implications

This source contributes Nigerian-market beverage occurrence data for total arsenic and total chromium in canned and non-canned beverages. It is relevant to broad beverage routing, including soft drinks, fruit drinks/juices, soy-milk beverages, and milk beverages, but it should not be used for brand ranking or for chromium speciation. The values support category-level contamination context and source retrieval for later structured beverage extraction.

Verification notes

  • PDF text extracted with pdftotext -layout; title page, abstract, methods, Tables 1-2, discussion, and references were readable.
  • No DOI was printed in the extracted source text; doi is left null and no_doi_assigned is set true. Raw-handle, title/author, and cite-key checks found no existing primary source page before creation, though the later Izah 2016 Nigerian-beverage review cites this paper as secondary context.
  • All aggregate ranges, sample counts, exceedance percentages, MCL comparator values, detection limit, wavelengths, and digestion details were checked against the extracted abstract, Results text, Methods section, and table footnotes.
  • Units are preserved as reported (mg/L); no conversion to µg/L or ppb was performed.
  • Speciation: arsenic is reported as arsenic after nitric-acid digestion and AAS, so it is labeled total arsenic (tAs) in frontmatter. Chromium is reported as total chromium (Cr), not Cr-VI.
  • Brand firewall: the source’s tables attach commercial drink names to As/Cr values. This page intentionally omits all drink names from Key numbers and reports only aggregate ranges and exceedance percentages.
  • Frontmatter product and ingredient slugs were checked against docs/gpt-collaboration/taxonomy-snapshot.md; no new product or ingredient slug was invented.

Page history

The five most recent substantive edits to this page. The full version history lives in git; when DOI minting comes online (see schema docs), each entry below will also link to a version-pinned DataCite DOI.

CommitDateDescription
97920102026-06-08ingest: garrity1990-mt1-tissue-specific-promoter fresh from MFK/heavy_metals_peptides