Marinescu et al. 2020 - Romanian herbs and spices metals
Marinescu et al. measured arsenic, cadmium, copper, iron, mercury, and lead in 42 Romanian medicinal-plant and culinary herb/spice samples. The spice subset covers dill, marjoram, oregano, peppermint, parsley, and thyme, with packaged samples and spontaneous-flora samples. The source is routeable occurrence evidence for herbs/spices and herbal-tea matrices, but packaged and wild-growing samples should not be silently pooled because the authors observed higher cadmium in spontaneous-flora spice samples.
Key numbers
Tables III and IV report mean +/- standard deviation in mg/kg. Selected spice values from Table IV:
| Spice/sample group | tAs | Cd | Cu | Fe | tHg | Pb |
|---|---|---|---|---|---|---|
| Dill, AG1 packaged | 0.04 | 0.02 | 127 | 320 | ND | 0.09 |
| Dill, AG2 packaged | ND | 0.04 | 142 | 348 | ND | 0.08 |
| Dill, AG3 wild-growing | 0.08 | 0.12 | 133 | 320 | ND | ND |
| Marjoram, OM1 packaged | ND | ND | 163 | 657 | ND | 0.14 |
| Marjoram, OM2 packaged | 0.01 | 0.05 | 131 | 719 | ND | 0.13 |
| Marjoram, OM3 wild-growing | 0.07 | 0.05 | 348 | 473 | ND | 0.95 |
| Oregano, OV1 packaged | 0.03 | 0.06 | 201 | 1375 | 0.374 | ND |
| Oregano, OV2 packaged | 0.21 | 0.06 | 198 | 1460 | 0.019 | 0.04 |
| Oregano, OV3 wild-growing | 0.33 | 0.07 | 222 | 2471 | 0.075 | ND |
| Peppermint, MP1 packaged | 0.18 | 0.01 | 309 | 6683 | ND | 0.58 |
| Peppermint, MP2 packaged | 0.09 | 0.05 | 237 | 2378 | ND | 0.18 |
| Peppermint, MP3 wild-growing | ND | 0.10 | 157 | 673 | 0.010 | 1.28 |
| Parsley, PC1 packaged | 0.78 | ND | 133 | 1360 | 0.083 | 0.06 |
| Parsley, PC2 packaged | 0.19 | 0.05 | 122 | 336 | 0.052 | ND |
| Parsley, PC3 wild-growing | ND | 0.07 | 123 | 748 | 0.026 | 0.11 |
| Thyme, TV1 packaged | 0.03 | 0.03 | 191 | 1314 | 0.131 | 0.07 |
| Thyme, TV2 packaged | 0.42 | 0.07 | 131 | 1449 | 0.036 | 0.09 |
| Thyme, TV3 wild-growing | ND | 0.09 | 169 | 2578 | 0.024 | 0.11 |
Across the spice subset, the authors summarize arsenic as less than 0.01-0.78 mg/kg and cadmium as 0.02-0.12 mg/kg. Mercury exceeded the European Pharmacopoeia 0.1 mg/kg comparator in oregano OV1 (0.374 mg/kg) and thyme TV1 (0.131 mg/kg). Lead exceeded the EU 0.3 mg/kg comparator in some samples, including wild-growing marjoram (0.95 mg/kg) and wild-growing peppermint (1.28 mg/kg).
Methods (brief)
The authors analyzed 42 samples from six medicinal plant species and six spice species commonly used in Romania. Heavy metals were measured after wet digestion with 65% nitric acid and 30% hydrogen peroxide. Arsenic, cadmium, and lead were measured by graphite-furnace atomic absorption spectrometry; copper and iron by flame atomic absorption spectrometry; and mercury by cold-vapour atomic absorption spectrometry. Four determinations were performed for each sample.
Implications
Certification: The spice subset provides occurrence evidence for total arsenic, cadmium, mercury, and lead in Romanian culinary herbs/spices, with important separation between packaged and spontaneous-flora samples.
Courses: The source is useful for teaching that medicinal-plant and culinary-herb markets overlap; route herbal-tea and spice implications separately.
App: Broad herbs-and-spices routing is appropriate for most species. Parsley can route to the existing parsley ingredient page.
Microbiome (if applicable): The paper does not study microbiome outcomes.
Wiki pages this source may touch
Verification notes
The PDF title, byline, DOI, year, journal, sample descriptions, methods, and Tables III-IV values were read from the auto-fetched PDF. The paper reports element names without arsenic or mercury speciation, so arsenic and mercury are treated as total-element occurrence evidence. Packaged and wild-growing samples are source-distinct and should not be pooled without a logged basis decision. Matrix note: spices is a controlled matrix-map label; medicinal-plants and herbal-teas are source-scope descriptors retained to separate the medicinal-plant/herbal-tea portion of the source from the culinary-spice subset.
Page history
The five most recent substantive edits to this page. The full version history lives in git; when DOI minting comes online (see schema docs), each entry below will also link to a version-pinned DataCite DOI.
| Commit | Date | Description |
|---|---|---|
| a79beff | 2026-06-03 | ingest auto-fetched 2026-06-03: pradhan2023-heracleum-nepalense-elements |